EUV and soft X-ray photoelectron spectroscopy of isolated atoms and molecules using single-order laser high-harmonics at 42 eV and 91 eV

Papers published
Mizuho Fushitania, Akitaka Matsudaa, Akiyoshi Hishikawa, J. Electron. Spectrosc. Relat. Phenom.2012, in press. DOI:10.1016/j.elspec.2011.10.002
  • Photoelectron spectroscopy of isolated atoms and molecules using single-order high-harmonics of Ti:Sapphire laser pulses (800nm, 12fs/30fs) is demonstrated. Dielectric multilayer mirrors, SiC/Mg and Mo/Si, are used to isolate the 27th (42eV) and 59th (91eV) order harmonics, respectively. The obtained harmonics are characterized by valence and inner-shell photoelectron spectroscopy of Xe. The applications to two-color two-photon ionization of He and pump-probe spectroscopy of ultrafast photodissociation of Br2 , Br2 (C1

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