An Ambipolar Conducting Covalent Organic Framework with Self-Sorted and Periodic Electron Donor-Acceptor Ordering

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Xiao Feng, Long Chen, Yoshihito Honsho, Oraphan Saengsawang, Lili Liu, Lu Wang, Akinori Saeki, Stephan Irle, Shu Seki, Yuping Dong, Donglin Jiang Adv. Mater. 24, 3026-3031 2012, DOI: 10.1002/adma.201201185
  • A donor-acceptor built-in covalent organic framework with segregated, periodic, and bicontinuous electron donor-acceptor ordering is reported. The framework consists of pre-organized periodic independent pathways for ambipolar electron and hole conduction and constitutes vertically ordered p-n heterojunctions with a broad D-A interface for enhanced photoconductivity.

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